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ZnTe Augments Broadband Terahertz Radiation

A THz emitter just 40 nm thick can perform as well as much thicker traditional emitters
Metamaterials scientists at the U.S. Department of Energy's Ames Laboratory have demonstrated broadband terahertz (THz) wave generation using metamaterials.

The metamaterial is based on zinc telluride (ZnTe).

ZnTe can be easily doped, and for this reason it is one of the more common compound semiconducting materials used in optoelectronics.

The material is important for development of various semiconductor devices, including blue LEDs, laser diodes, solar cells, and components of microwave generators. It can be used for solar cells, for example, as a back-surface field layer and p-type semiconductor material for a CdTe/ZnTe structure or in PIN diode structures.

The material can also be used as a component of ternary semiconductor compounds, such as CdxZn(1-x)Te (conceptually a mixture composed from the end-members ZnTe and CdTe), which can be made with a varying composition x to allow the optical bandgap to be tuned as desired.



A THz spectrometer driven by femtosecond laser pulses was used to demonstrate THz emission from a split-ring resonator metamaterial of single nanometre thickness

The discovery may help develop non-invasive imaging and sensing, and make possible THz-speed information communication, processing and storage. The results appeared in the January 8th issue of Nature Communications.

Terahertz electromagnetic waves occupy a middle ground between electronics waves, like microwave and radio waves, and photonics waves, such as infrared and UV waves.

Potentially, THz waves may accelerate telecom technologies and break new ground in understanding the fundamental properties of photonics. Challenges related to efficiently generating and detecting THz waves has primarily limited their use.

Traditional methods seek to either compress oscillating waves from the electronic range or stretch waves from the optical range. But when compressing waves, the THz frequency becomes too high to be generated and detected by conventional electronic devices.

So, this approach normally requires either a large-scale electron accelerator facility or highly electrically-biased photoconductive antennas that produce only a narrow range of waves.

To stretch optical waves, most techniques include mixing two laser frequencies inside an inorganic or organic crystal. However, the natural properties of these crystals result in low efficiency.

So, to address these challenges, the Ames Laboratory team looked outside natural materials for a possible solution. They used man-made materials called metamaterials, which exhibit optical and magnetic properties not found in nature.

Costas Soukoulis, an Ames Laboratory physicist and expert in designing metamaterials, along with collaborators at Karlsruhe Institute of Technology in Germany, created a metamaterial made up of a special type of meta-atom called split-ring resonators. Split-ring resonators, because of their u-shaped design, display a strong magnetic response to any desired frequency waves in the THz to infrared spectrum.



A team led by Ames Laboratory physicists demonstrated broadband, gapless terahertz emission (red line) from split-ring resonator metamaterials (background) in the telecomm wavelength. The THz emission spectra exhibit significant enhancement at magnetic-dipole resonance of the metamaterials emitter (shown in inset image). This approach has potential to generate gapless spectrum covering the entire THz band, which is key to developing practical THz technologies and to exploring fundamental understanding of optics

Ames Laboratory physicist Jigang Wang, who specializes in ultra-fast laser spectroscopy, designed the femto-second laser experiment to demonstrate THz emission from the metamaterial of a single nanometre thickness.

“The combination of ultra-short laser pulses with the unique and unusual properties of the metamaterial generates efficient and broadband THz waves from emitters of significantly reduced thickness," says Wang, who is also an associate professor of Physics and Astronomy at Iowa State University.

The team demonstrated its technique using the wavelength used by telecommunications (1.5 µm), but Wang says that the THz generation can be tailored simply by tuning the size of the meta-atoms in the metamaterial.

“In principle, we can expand this technique to cover the entire THz range," says Soukoulis, from Iowa State University.

What’s more, the team’s metamaterial THz emitter measured only 40 nm thick and performed as well as traditional emitters that are thousands of times thicker.

“Our approach provides a potential solution to bridge the ‘THz technology gap’ by solving the four key challenges in the THz emitter technology: efficiency; broadband spectrum; compact size; and tunability," adds Wang.

This work is partially supported by Ames Laboratory’s Laboratory Directed Research and Development (LDRD) funding.

This research has been published in the paper, "Broadband terahertz generation from metamaterials," by Liang Luo et al in Nature Communications,5, (3055).  DOI:10.1038/ncomms4055



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